Chromium OS vs NixOS
When comparing Chromium OS vs NixOS, the Slant community recommends NixOS for most people. In the question“What are the best Linux distributions for desktops?” NixOS is ranked 19th while Chromium OS is ranked 89th. The most important reason people chose NixOS is:
Atomic non-destructive upgrades / rollback of a system upgrade / declarative reproducible system configuration / unprivileged installation of packages / transparent source or binary deployment.
Specs
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Pros
Pro Safe and requires little to no maintenant
Since you only have the browser, you cannot install applications (outside Chrome Apps which are decently protected by their limited API and the Chrome Web Store). This means no harmful virus, and also nearly no way you can screw your system. Everything will just work.
Pro Minimalistic interface
Chromium's system UI uses as little screen space as possible by combining apps and standard web pages into a minimal tab strip: While existing operating systems have web tabs and native applications in two separate strips, Chromium OS combines these, giving access to everything from one strip. The tab is the equivalent of a desktop application's title bar; the frame containing the tabs is a simple mechanism for managing sets of those applications and pages.
Pro Lightweight
Because Chromium OS is designed for users who spend most of their computer time on the Web, it is intended for use in computers with little local storage and fast boot-up times.
Pro State of the art package manager
Atomic non-destructive upgrades / rollback of a system upgrade / declarative reproducible system configuration / unprivileged installation of packages / transparent source or binary deployment.
Pro Minimal
You can start with a minimal environment and add packages and software to suit your needs as you go along.
Pro Reproducible system
NixOS is configured using the Nix package manager, allowing your system to be replicated and kept in sync across multiple machines. Great for keeping a laptop and desktop in sync.
Pro Robust
Packages don't break after a NixOS upgrade as they are prone to with other distros (especially Arch).
Cons
Con Google
Possibly harms your privacy.
Con Made for developers
ChromiumOS is mainly made for development, so there exist no official install images and you have to build it from source or use third party images like Arnold's or the waterfall images.
Con No auto-upgrade (unlike Chrome OS)
Chrome OS auto-upgrade the system, but Chromium OS does not. It's possible that they're thinking about adding that feature from the design doc.
Con Documentation is not good
A lot of the documentation of various functions is buried on the source code, their respective manuals, or non-existent. The documentation, the conventions, and the scattered toolchain really made searching for stuff easily missable.