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VLC is a media player first and foremost. There is no library management, aside from playlists, usage of tags is very limited, no rating system and VLC is best at playing a file directly from a folder as opposed to helping you manage or find good songs in your music library. See More
The interface of iTunes presents a flat, clean design with playback controls at the top-left, search at the top-right, and a row of ways to categorize available media beneath that. It can also be minimized to take up much less space. The minimized interface is called the Mini Player and it can be set to display on top of all other windows. It's possible to show iTunes on top of all other windows when playing movies as well. See More
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